发表论文 - 蒋 臣威
论文标题 | Selective control of vibrational modes with sequential femtosecond-scale laser pulses. |
作者 | Chen-Wei Jiang, Rui-Hua Xie, Fu-Li Li et al. |
发表/完成日期 | 2011-11-01 |
期刊名称 | Chemical Physics Letters |
期卷 | 515 |
相关文章 | |
论文简介 | For nonresonant femtosecond-scale laser pulses, we showed earlier that the optimum FWHM pulse duration is 0.42 T if one wishes to achieve maximum relative excitation of a specific vibrational mode with period T. Here we show that much greater enhancement of a specific mode can be achieved with a sequence of laser pulses which have both this optimized duration and optimized delays between pulses. One can thus enhance a selected set of modes that are particularly useful in identifying or characterizing a chemical system, to lift them out of the background of less informative modes. |